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<article xmlns:xlink="http://www.w3.org/1999/xlink">
  <front>
    <journal-meta />
    <article-meta>
      <title-group>
        <article-title>Nonlinear Finite Element Simulation of Thin Dielectric Elastomer Structures</article-title>
      </title-group>
      <contrib-group>
        <contrib contrib-type="author">
          <string-name>Sandro Zwecker</string-name>
          <email>1zwecker@rhrk.uni-kl.de</email>
        </contrib>
        <contrib contrib-type="author">
          <string-name>Sven Klinkel</string-name>
          <email>2klinkel@rhrk.uni-kl.de</email>
        </contrib>
        <contrib contrib-type="author">
          <string-name>R. Müller</string-name>
          <xref ref-type="aff" rid="aff0">0</xref>
        </contrib>
        <contrib contrib-type="author">
          <string-name>Statik und Dynamik der Tragwerke</string-name>
        </contrib>
        <contrib contrib-type="author">
          <string-name>TU Kaiserslautern Paul-Ehrlich-Str.</string-name>
        </contrib>
        <contrib contrib-type="author">
          <string-name>Kaiserslautern</string-name>
        </contrib>
        <contrib contrib-type="author">
          <string-name>Germany</string-name>
        </contrib>
        <aff id="aff0">
          <label>0</label>
          <institution>Lehrstuhl für Technische Mechanik</institution>
          ,
          <addr-line>TU Kaiserslautern Postfach 30 49, 67653 Kaiserslautern</addr-line>
          ,
          <country country="DE">Germany</country>
        </aff>
      </contrib-group>
      <abstract>
        <p>- To simulate the behavior of thin dielectric elastomer structures a finite solid shell element formulation is presented. Dielectric elastomers belong to the group of electroactive polymers and their use as actuators is caused by the efficient coupling between electrical energy input and mechanical energy output. Also the large elongation strain of 120-380% of the dielectric elastomer actuators and their light weight are advantages that make the material very attractive. Regarding the electro-mechanical coupling a constitutive model is expounded. For the definition of an electric stress tensor and a total stress tensor the electrical body force and couple are considered in the balance of linear momentum and angular momentum, respectively. The governing constitutive equations are derived and incorporated in a solid shell element formulation based on a Hu-Washizu mixed variational principle considering six fields: displacements, electric potential, strains, electric field, mechanical stresses, and dielectric displacements. This formulation allows large deformations and accounts for physical nonlinearities to capture the main characteristics of dielectric elastomers.</p>
      </abstract>
    </article-meta>
  </front>
  <body>
    <sec id="sec-1">
      <title>I. INTRODUCTION</title>
      <p>In recent years dielectric elastomers (DE) have become
popular for the usage in actuators. The efficient
transformation of electrical energy in mechanical energy and
the ability to maintain large strains makes them very attractive.
A Constitutive model, which describes the specific material
behavior, is introduced by Dorfmann and Ogden [1],
Steigmann [2] and the references therein. The numerical
treatment in the context of the finite element method is
presented by Vu et al. [3], who provide a brick element
formulation, which incorporates the nonlinear constitutive
model. In the present work a shell finite element formulation
for DE is presented. It is motivated by the fact that the most
DE devices are thin structures, which have a very high length
to thickness ratio. The electromechanical coupling is
considered in the body force and the couple density, see e.g.
Eringen and Maugin [4] or Müller et al. [5]. The angular
momentum equation is fulfilled by assuming a Maxwell stress
tensor. The linear momentum equation is approximately
fulfilled by the finite element method. A mixed solid shell
element formulation is introduced. It incorporates specific
interpolations for the displacements, strains, stresses as well as
for the electric potential, electric field and dielectric
displacements. As nodal degrees of freedom three
displacements and the electric potential are assumed. The
mixed formulation allows for a consistent finite element
approximation to avoid electromechanical locking effects. The
element formulation is able to simulate large deformations.
Some numerical examples show the applicability of the
proposed solid shell element.</p>
    </sec>
    <sec id="sec-2">
      <title>II. KINEMATICS</title>
      <p>Let Φ be a deformation that point maps ⃗⃗ of the reference
configuration to ⃗ of the current configuration at time ,
see Figure 1. The deformation gradient is declared as the
tangent to Φ and given by</p>
      <p>With this definition for the deformation gradient the right</p>
    </sec>
    <sec id="sec-3">
      <title>Cauchy-Green deformation tensor reads, Followed by the Green-Lagrange strain tensor defined as</title>
      <p>⃗⃗ .
(3)</p>
      <p>To describe the shell formulation convective coordinates
are introduced, where and are the in-plane coordinates
and is the coordinate in thickness direction. The covariant
contravariant basis vectors are defined in a standard manner
by ⃗⃗ ⃗⃗ and ⃗⃗ ⃗⃗ , where is the
Kroneckerdelta. With this convective description the deformation
gradient also reads ⃗⃗ ⃗⃗ .</p>
      <p>A potential is used to describe the electric field ⃗ . With
satisfying the Laplace’s equation ⃗ reads
⃗ (⃗ ) ⃗ (⃗ )
order terms results in
by neglecting higher
⃗
(∑
) ⃗
(∑
) ⃗
,
⃗ - (∑
⃗
) .
⃗
by</p>
      <p>Applying the pull-back operation the physical electric field
⃗ is observed. The displacement vector ⃗ is defined</p>
    </sec>
    <sec id="sec-4">
      <title>Boundary conditions for ⃗ and</title>
      <p>, respectively.
are given on</p>
    </sec>
    <sec id="sec-5">
      <title>III. FORCE AND COUPLE DENSITY</title>
      <p>To get a macroscopic representation of force and couple
density a close look on the microscopic level is presented.
Therefore the physical model will start with a particle of
the current configuration to deduce electric force in the
presence of electromagnetic matter and in absence of a
magnetic field.
⃗
⃗
⃗
⃗</p>
      <p>⃗ .
(4)
(5)
and
∫ ⃗
∫
,
⃗
⃗
⃗</p>
      <p>⃗⃗ .
⃗
⃗⃗ .</p>
      <p>After defining the resultant mass ∑ , charge
∑ , and polarization ⃗ ∑ ⃗ of the particle
and performing a simple space averaging ∑ ,
∑ , ⃗ ∑ ⃗ leads to the macroscopic body
force density
⃗
⃗
⃗
,
⃗
⃗
⃗ ,
where ⃗ combines the electric contribution to the body
force density. Deriving the corresponding couple density with
the same arguments the resultant couple of the particle
with respect to the mass center reads
∑ ⃗
⃗
∑ ⃗
⃗ .</p>
      <p>Here it is assumed that the mass dipole moment
∑ ⃗ ⃗ . With the resultant polarization ⃗
∑ ⃗ and a space averaging it follows the macroscopic
couple density</p>
      <p>Relative to the mass center eccentric by ⃗ not to be
confused with the convective coordinates are the point
charges and the point masses , as shown in Figure 2.
In an electric field a force is acting on each point charge
called Lorentz force and it is defined by ⃗ . The
gravitation field ⃗ is acting on each point mass producing the
Newton force given by ⃗ . Summing over leads to the
resultant force on the particle:
∑
⃗</p>
      <p>The position of a point within the particle can be
described by ⃗ ⃗ ⃗ . Assuming the gravitation to
be constant it follows: ⃗ (⃗ ) ⃗ (⃗ ). This assumption and
expanding the external field in a Taylor series
(7)
(8)
(9)
(10)
(11)
(12)
(13)</p>
    </sec>
    <sec id="sec-6">
      <title>IV. BALANCE LAWS AND STRESS TENSOR</title>
      <p>The balance laws incorporating the electric force, couple,
and power densities are summarized. After that the global
integral forms and the local field equations are presented. The
Cauchy stress tensor and an electric stress tensor are
introduced. Conservation of mass ∫ , with
is assumed. Localization of the material description
results in . In quasi static processes the integral form
of the balance of linear momentum is given as</p>
      <p>where ⃗ is the body force density (8) and the traction
vector on . With the Cauchy stress tensor the traction is
determined by a linear map of the normal vector ⃗ ,
according to Cauchy’s stress theorem. Considering
conservation of mass, applying the divergence theorem and
the localization theorem, the field equation along with the
jump condition are observed as
⃗
⃗
⃗
⃗
on
in</p>
      <p>With as a prescribed traction on the boundary . The
boundaries with a given traction and a given displacement
satisfy ⋃ and ⋂ . The global
form of the balance of angular momentum reads
∫ ⃗
⃗
∫
⃗
where ⃗ is the couple density Using the integral
theorem, considering conservation of mass and the linear
momentum balance along with the localization theorem
results in the field equation
⃗</p>
      <p>For dielectric materials the conservation of charge in
integral form with the surface charge density on reads</p>
      <p>The dielectric displacement vector is denoted by ⃗ and
determined by Gauss’ law ⃗ ⃗ . Applying the
divergence theorem results in the field equation along with the
jump condition
⃗ .</p>
      <p>,</p>
    </sec>
    <sec id="sec-7">
      <title>V. CONSTITUTIVE EQUATIONS</title>
      <p>Introducing the energy function
(⃗
⃗ )
[(⃗
⃗ )
where is a function of to fulfill material objectivity,
here an Ogden-type material is chosen, and the susceptibility
of the material is denoted by , the total stress and the
dielectric displacements are derived as
⃗
⃗
⃗
⃗
(
⃗
⃗
⃗
, (
⃗⃗
⃗⃗</p>
      <p>⃗
⃗⃗ ⃗⃗</p>
      <p>Here, is a prescribed surface charge. For the total
boundaries with a given electric potential and a given surface
charge it holds ⋃ and ⋂ .
With the constitutive equations in matter the dielectric
displacements are given as ⃗ ⃗ ⃗ , where is the
permittivity in vacuum and the polarization depends on the
considered material. An electric stress tensor is introduced as
such that
⃗ ⃗
⃗ and</p>
      <p>⃗ . It is remarked that
is also known as Maxwell stress tensor.</p>
      <p>With  it follows that the total stress tensor has to be
symmetric. The remaining field equations and boundary
conditions are
⃗</p>
      <p>⃗
⃗ ⃗
)
⃗
⃗
⃗
⃗
⃗ ⃗
,
(19)
Considering the 2nd Piola-Kirchhoff stress tensor
and , the pull-back of the dielectric displacement
⃗⃗ ⃗ and the transformation of the densities by leads
to the material description
)⃗
⃗
on</p>
      <p>in
on
on
in
in
on
on
in
in</p>
      <p>Where ⃗ is the traction with respect to the reference
configuration.</p>
      <p>,</p>
      <p>In this section a mixed variational formulation is introduced.
Let the set { ⃗ , ( )- ⃗ ⃗ } be the space of
admissible displacement variations and { , (
)} be the space of admissible electric potential
variations. Further let * , ( )- + , *
, ( )- + the spaces of admissible variations of the total
stresses and strains and { ⃗⃗ , ( )- } , { ⃗ , ( )- }
the spaces of admissible variations of the dielectric
displacement and the electric field. Since the variations are
arbitrary the field equations (24)-(27), the constitutive
equations (29), (20), and the kinetic field equations (3), (4) are
rewritten as
Applying integration by part, using the divergence theorem and
considering the boundary conditions the weak formulation
reads
)⃗ )</p>
      <p>⃗
)
))
⃗
⃗⃗
)) (
,
,
⃗
(</p>
      <p>∫
⃗
⃗⃗ ⃗
) (
⃗ ⃗
)
(
⃗⃗</p>
      <p>)
)
⃗
⃗⃗
with
⃗ ,</p>
      <p>In this section a solid shell element is introduced. The finite
element approximation is constructed in the sense that the
whole domain is divided in element domains with
⋃ , where is the total number of elements. The
geometry, displacements, and electric potential are
approximated as ⃗⃗ ∑ ⃗⃗ , ⃗ ∑ ⃗ , and
∑ with the same interpolation functions
( )( )( ) , at
nodes . The vectors ⃗⃗ and ⃗ contain the nodal
coordinates and displacements, respectively. Arranging in
the matrix , - with
, - , the virtual quantities are
interpolated as
[
⃗
]</p>
      <p>⃗ ,
where ⃗ [⃗ ⃗ ⃗ ⃗ ] is the vector of nodal
degrees of freedom ⃗ ,⃗ ⃗ ⃗ - .</p>
    </sec>
    <sec id="sec-8">
      <title>Accordingly, ⃗ is the vector of the virtual values.</title>
      <p>The gradient fields are defined with respect to the curvilinear
coordinates . The constitutive equations  and  will
be given with respect to a local orthonormal coordinate system
⃗ . This necessitates a transformation of the strains and the
electric field. Introducing the transformation matrix</p>
      <p>The approximation on element level of the virtual gradient
field ⃗ reads
defined with
⃗ ⃗
‖⃗ ⃗ ‖
where</p>
      <p>⃗
and ⃗ ‖⃗ ‖ , ⃗ , ⃗ ⃗ ⃗ . The Jacobian
matrix is denoted by ⃗⃗ ⃗ . For the sake of a compact
notation the contravariant components of the virtual strain
tensor and the virtual electric field vector are arranged in a
generalized vector
,
and
⃗
Quantities, which are evaluated at the element center are
denoted with the index and is a identity matrix. The
transformation matrix is obtained by  considering
and . The matrices and ⃗ are defined as
- and
[
is defined with some ANS interpolations in [6]
⃗ /
⃗ /
(
(
⃗
)
) .
) .</p>
      <p>⃗
⃗
⃗
- .
where denotes the partial derivative of the shape function
with respect to the curvilinear coordinates. The matrix at
the node is determined as
The physical stresses and dielectric displacements are derived
from the potential function and are arranged in the vector
0 ⃗ ⃗ ⃗ ⃗ 1 . Here, ⃗ are independently
assumed quantities for strain and electric field components and
are approximated with the following interpolations, see Klinkel
and Wagner [7]:
⃗</p>
      <p>⃗⃗ ,
with
⃗⃗</p>
      <p>⃗
. The matrices
] ,
and
[</p>
      <p>⃗
⃗ are given as
] , ⃗⃗</p>
      <p>,
with
The matrix
and reads</p>
      <p>(
[
( )
,
⃗⃗
( )
,
⃗ /</p>
      <p>] .

]

The approximation of the independent field
is defined as
with
The weak formulation of  will be approximated on
element level as following:
,
with</p>
      <p>. In Eq. (59) the body and surface
loads are determined by ⃗̃
, ⃗
- and ̃
0⃗</p>
      <p>Having in mind that (50) is solved iteratively the following
approximation on element level is obtained
,
⃗ ⃗
⃗
⃗</p>
      <p>⃗
)
)
⃗
⃗
,
⃗ ⃗
⃗ ⃗ ⃗
⃗ 
⃗ ⃗</p>
      <p>⃗⃗ ,
∫
∫
∫
∫
∫
+∫
∫ (
∫ (
∫
∫
∫ (
∫
⃗
⃗
,
⃗
⃗⃗
⃗⃗
⃗⃗
∫
∫
and
⃗
⃗
⃗
⃗</p>
      <p>⃗
⃗</p>
      <p>⃗ ,


⃗







⃗
⃗
⃗
] [ ⃗ ])


Taking into account that the finite element interpolations for
the fields ⃗ and ⃗ are discontinuous across the element
boundaries a condensation on element level yields the element
stiffness matrix and the right hand side vector
with the unknown incremental nodal displacements and the
electric potential. The update of the internal degrees of
freedom reads
,
⃗
⃗ ,
with ⃗ , ⃗ - and ⃗ contains the components of ,
, and ⃗⃗ accordingly to the vector notation. The weak form is
solved iteratively by employing Newton-Raphson’s method.
This requires the linearization
with</p>
      <p>(
⋃
obtains</p>
      <p>( ) and ⃗
) ⃗ . After assembly over all elements
, ⃗ ⋃ ⃗ and ⃗ ⋃ ⃗
one
Considering the above interpolations  and  one obtains
the following matrices:
where</p>
      <p>is the matrix of [7] and vectors
⃗
⃗
) .
(⃗
⃗</p>
      <p>⃗ /
⃗ )
, and .</p>
      <p>The relative permittivity is given as ( ) .</p>
      <p>In Table 1 it is shown that there is only eigenvalue number
18 much greater than zero. This eigenvalue accounts for the
volumetric locking mode which arises by incompressible
materials like DE. At this point no other locking modes are
observed. The result is also the same when taking an irregular
non-cube element.
B. Bending Actuator</p>
      <p>The second example is presented to demonstrate the valid
reflection of the electro-mechanical coupling phenomenon of
DEs. Therefore a square plate with the dimension of
is investigated. It is clamped on one side
and consists of two layers with the thickness of each,
see Figure 3. The dataset of the material is the same as given
in the first example.</p>
      <p>To get a bending answer of the thin structure either the
upper or lower layer is loaded by an electric field applied in
thickness direction of the structure. Due to the
electromechanical coupling the loaded layer responds with an
inplane extension. Because of the eccentricity the bending effect
of the whole structure occurs. Figure 4 shows several
deformed configurations.</p>
      <p>Fig. 4 Bending actuator - several deformed configurations
In the simulation the surface charge is increased from to
and decreases back to again. Then the other
layer is loaded in the same way. The tip deflection versus the
applied voltage is shown in Figure 5.</p>
      <p>80
60
-60
-80
1000
2000
3000
4000
5000
6000</p>
      <p>7000</p>
      <p>Load j [V]</p>
    </sec>
    <sec id="sec-9">
      <title>IX. SUMMARY AND OUTLOOK</title>
      <p>The presented element formulation is based on a mixed
variational approach. It results in an independent interpolation
of the displacement, electric potential, strains, electric field,
stresses and dielectric displacements. The element possesses
only four nodal degrees of freedom, displacements and the
electric potential. It allows a consistent approximation of the
electromechanical coupled problem. The governing field
equations and boundary conditions are presented. The
formulation accounts for geometric and material nonlinear
behavior. Further tasks will be to embed the material
formulation into an improved stabilized element formulation.
For more accurate simulations other material models for the
mechanical part should be discussed.</p>
    </sec>
    <sec id="sec-10">
      <title>ACKNOWLEDGMENT</title>
      <p>We want to thank the Landesforschungszentrum CM² for
financially supporting our project Mikro- &amp; Strukturmechanik
zur Analyse des nichtlinearen Deformationsverhaltens von
dielektrischen und porösen Elastomeren (MSADEL).</p>
    </sec>
  </body>
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